资源化学领域

简历:

甄文龙,男,1988年10月生,中国科学院兰州化学物理研究所研究员,博士生导师。2016年博士毕业于兰州大学化学化工学院物理化学专业,师从马建泰教授,后于2016.06至2018.06在中国科学院兰州化学物理研究所吕功煊研究员课题组开展博士后研究,2018.07至2021.08在新加坡南洋理工大学薛灿副教授团队从事博士后研究,于2021年11月入职中国科学院兰州化学物理研究所。主要从事太阳能驱动光催化水分解制氢、二氧化碳催化转化以及环境催化等研究。现主持中国科学院“引才计划”青年项目(B类)、国家自然科学基金青年项目、甘肃省自然科学基金项目、研究所特聘青年研究员人才项目、研究所青年联盟合作基金项目等7项,参与国家重点研发计划1项。目前已在Nat. Commun.,Appl. Catal. B,J. Catal.,J.Mater. Chem. A,Int. J. Hydrogen Energy等国际学术期刊发表论文44篇,被引用2401次,单篇文章最高引用356次,ESI Top1%高被引论文1篇。

研究方向:

1.光催化分解水制氢

2.二氧化碳催化转化

3.能源与环境纳米催化材料

4.可再生能源转化利用

承担科研项目:

1. 国家自然科学基金青年项目:具有抑制氢氧复合逆反应功能光催化剂表界面构筑研究,2024.01-2026.12,主持。

2. 中国科学院“引才计划”青年项目(B类): 绿氢制备与二氧化碳转化新技术,2024.01-2026.12,主持。

3. 甘肃省自然科学基金项目:光伏驱动辉光电离催化CO2制取CO反应系统研究,2022.10-2024.09,主持。

4. 研究所青年联盟合作基金项目:等离子体活化CO2催化转化制备CO和O2反应研究2023.01-2024.12,主持。

5. 研究所特聘青年研究员人才项目:分子功能化材料光助催化转化CO2的研究,2021.11-2026.11,主持。

代表论著:

[1] Tianshuo Sui,Jingbo Mu,Wenlong Zhen,Zhixiao Zhang,Aifeng Liu,Yanming Wang,Hongwei Che,Guangshuo Wang,Zengcai Guo. The property and mechanism of peroxymonosulfate activation boosted carbon cage encapsulated Mo2C/Bi2O2CO3 Z-scheme heterojunction for enhanced catalytic degradation and antibacterial activity. Separation and Purification Technology,2025,353,128186

[2] Zhengzhi Han,Xiaofeng Ning,Zhiquan Yin,Wenlong Zhen,Gongxuan Lu,Bitao Su. Enhancement of photocatalytic activity for overall water splitting by inhibiting reverse reactions and photocorrosion of C3N4 via modified with TiO2 thin layer. International Journal of Hydrogen Energy,2024,59,856-865.

[3] Bo Yang,Wenlong Zhen,Jiantai Ma,Gongxuan Lu. Corrosion inhibition and stability enhancement of cobalt phosphide in aqueous solution by coating TiO2 layer. International Journal of Hydrogen Energy,2024,48,36784-36794.

[4] Jiajun Sun,Wenlong Zhen,Can Xue. Magnetic template-assisted construction of 2D PCN/TiO2 heterostructures for efficient photocatalytic hydrogen generation. Applied Surface Science,2023,623,157131.

[5] Ting He,Wenlong Zhen,Yongzhi Chen,Yuanyuan Guo,Zhuoer Li,Ning Huang,Zhongping Li,Ruoyang Liu,Yuan Liu,Xu Lian,Can Xue,Tze Chien Sum,Wei Chen & Donglin Jiang. Integrated interfacial design of covalent organic framework photocatalysts to promote hydrogen evolution from water. Nature Communications,2023,14,329.

[6] Lei Zeng,JieWei Chen,Lixiang Zhong,Wenlong Zhen,Yee Yan Tay,Shuzhou Li,YangGang Wang,Limin Huang,Can Xue. Synergistic effect of Ru-N4 sites and Cu-N3 sites in carbon nitride for highly selective photocatalytic reduction of CO2 to methane. Applied Catalysis B: Environment and Energy,2022,307,121154.

[7] 赵建军,甄文龙,吕功煊.固体氧化物电解CO2技术现状与前景. 燃料化学学报,2022,50,1237-1258.

[8] 甄文龙,赵建军,吕功煊.等离子体电离耦合催化的研究进展. 化学研究与应用,2022,34,2585-2597

[9] Xu Yuan,Wenlong Zhen,Sijia Yu,Can Xue. Plasmon Coupling-Induced Hot Electrons for Photocatalytic Hydrogen Generation. Chemistry—An Asian Journal,2021,16,3683-3688

[10] Wenlong Zhen,Jiajun Sun,Xiaofeng Ning,Xiangyan Shi,Can Xue. Polymeric Carbon Nitride with Internal n-p Homojunctions for Efficient Photocatalytic CO2 Reduction Coupled with Cyclohexene Oxidation. Applied Catalysis B: Environmental,2021,298,120568.

[11] Zengcai Guo,Yuanxiang Zhao,Hongwei Shi,Xu Yuan,Wenlong Zhen,Lixin He,Hongwei Che,Can Xue,Jingbo Mu. MoSe2/g-C3N4 heterojunction coupled with Pt nanoparticles for enhanced photocatalytic hydrogen evolution. Journal of Physics and Chemistry of Solids,2021,156,110137

[12] Chunhui Dai,Ting He,Lixiang Zhong,Xingang Liu,Wenlong Zhen,Can Xue,Shuzhou Li,Donglin Jiang,Bin Liu. 2,4,6-Triphenyl-1,3,5-Triazine Based Covalent Organic Frameworks for Photoelectrochemical H2 Evolution. Advanced Materials Interfaces,2021,8,2002191.

[13] Wenlong Zhen,Can Xue. Atomic‐ and Molecular‐Level Functionalizations of Polymeric Carbon Nitride for Solar Fuel Production. Solar RRL,2021,5,2000440.

[14] Wenlong Zhen,Xu Yuan,Xiangyan Shi,Can Xue. Grafting Molecular Cobalt-oxo Cubane Catalyst on Polymeric Carbon Nitride for Efficient Photocatalytic Water Oxidation. Chemistry—An Asian Journal,2020,15,2480−2486.

[15] Yanan Wang,Wenlong Zhen,Yiqing Zeng,Shipeng Wan,Haiwei Guo,Shule Zhang,Qin Zhong. In situ Self-assembly of Zirconium Metal–organic Frameworks onto Ultrathin Carbon Nitride for Enhanced Visible Light-driven Conversion of CO2 to CO. Journal of Materials Chemistry A,2020,8,6034−6040.

[16] Wenlong Zhen,Xu Yuan,Xiaofeng Ning,Xuezhong Gong,Can Xue. Building Oxime-Ni2+ Complex on Polymeric Carbon Nitride: Molecular-Level Design of Highly Efficient Hydrogen Generation Photocatalysts. ACS Applied Materials & Interfaces,2020,12,868−876.

[17] Dan Luo,Qun Zheng,Zhengrong Zhang,Zhonghua Guo,Xiufang We,Wenlong Zhen,Xuqiang Zhang. Amide–induced monodispersed Pt(100) nanoparticles loaded on graphene surface for enhanced photocatalytic hydrogen evolution. International Journal of Hydrogen Energy,2019,44,28123-28133.

[18] Xiaofeng Ning,Wenlong Zhen,Xuqiang Zhang,Gongxuan Lu. Assembly of Ultra-Thin NiO Layer Over Zn1−xCdxS for Stable Visible-Light Photocatalytic Overall Water Splitting. ChemSusChem,2019,12,1410-1420.

[19] Gongxuan Lu,Xuqiang Zhang,Wenlong Zhen. The Detection of K-Ca Transmutation in the Mixture of K and Hydride Chemicals. Journal of Molecular Catalysis(China),2019,33,1-9.

[20] Meng Wang,Wenlong Zhen,Bin Tian,Jiantai Ma,Gongxuan Lu. The Inhibition of Hydrogen and Oxygen Recombination Reaction by Halogen Atoms on Over-all Water Splitting over Pt-TiO2 Photocatalyst. Applied Catalysis B: Environmental,2018,236,240−252.

[21] Wenlong Zhen,Xiaofeng Ning,Meng Wang,Yuqi Wu,Gongxuan Lu. Enhancing Hydrogen Generation via Fabricating Peroxide Decomposition Layer over NiSe/MnO2-CdS Catalyst. Journal of Catalysis,2018,367,269−282.

[22] Xiaofeng Ning,Wenlong Zhen,Yuqi Wu,Gongxuan Lu. Inhibition of CdS Photocorrosion by Al2O3 Shell for Highly Stable Photocatalytic Overall Water Splitting under Visible Light Irradiation. Applied Catalysis B: Environmental,2018,226,373−383.

[23] Wei Gao,Wenyan Zhang,Bin Tian,Wenlong Zhen,Yuqi Wu,Xuqiang Zhang,Gongxuan Lu. Visible Light Driven Water Splitting over CaTiO3/Pr3+-Y2SiO5/RGO Catalyst in Reactor Equipped Artificial Gill. Applied Catalysis B: Environmental,2018,224,553−562.

[24] Wenlong Zhen,Xiaofeng Ning,Baojun Yang,Yuqi Wu,Zhen Li,Gongxuan Lu. The Enhancement of CdS Photocatalytic Activity for Water Splitting via Anti-photocorrosion by Coating Ni2P Shell and Removing Nascent Formed Oxygen with Artificial Gill. Applied Catalysis B: Environmental,2018,221,243−257.

[25] 甄文龙,高海波,吕功煊,马建泰. 担载Rh量子点三维石墨烯催化剂可见光催化制氢. 无机化学学报,2018,34,20−32.

[26] Zhen Li,Bin Tian,Wenlong Zhen,Wenyan Zhang,Xuqiang Zhang,Yuqi Wu and Gongxuan Lu. Enhancing Photoactivity for Hydrogen Generation by Electron Tunneling via Flip-flop Hopping over Möbius Strip-like RGO. Applied Catalysis B: Environmental,2017,219,501−510.

[27] Wenlong Zhen,Feng Gao,Bin Tian,Ping Ding,Yibing Ding,Zhen Li,Haibo Gao,Gongxuan Lu. Enhancing Activity for Carbon Dioxide Methanation by Encapsulating (111) Facet Ni Particle in Metal–Organic Frameworks at Low Temperature. Journal of Catalysis,2017,348,200–211.

[28] Wenlong Zhen,Wenjun Jiao,Yuqi Wu,Huanwang Jing,Gongxuan Lu. The Role of Interlayer Metallic Copper for Visible Photocatalytic Hydrogen Generation over Cu/Cu2O/Cu/TiO2 Catalyst. Catalysis Science & Technology,2017,7,5028−5037.

[29] Wenlong Zhen,Yueping Guo,Yuqi Wu,Gongxuan Lu. Co–P/graphene Alloy Catalysts Doped with Cu and Ni for Efficient Photocatalytic Hydrogen Generation. New Journal of Chemistry,2017,41,13804−13811.

[30] Bin Tian,Zhen Li,Wenlong Zhen,Xuqiang Zhang and Gongxuan Lu. Fe2S2 Nano-clusters Catalyze Water Splitting by Removing Formed Oxygen using Aid of an Artificial Gill under Visible Light. Journal of Catalysis,2017,352,572−578.

[31] Xiaofeng Ning,Jian Li,Baojun Yang,Wenlong Zhen,Zhen Li,Bin Tian,Gongxuan Lu. Inhibition of Photocorrosion of CdS via Assembling with Thin Film TiO2 and Removing Formed Oxygen by Artificial Gill for Visible Light Overall Water Splitting. Applied Catalysis B: Environmental,2017,212,129−139.

[32] Xuqiang Zhang,Bin Tian,Wenlong Zhen,Zhen Li,Yuqi Wu and Gongxuan Lu. Construction of Möbius-strip-like Graphene for Highly Efficient Charge Transfer and High Active Hydrogen Evolution. Journal of Catalysis,2017,354,258−269.

[33] Haibo Gao,Wenlong Zhen,Jiantai Ma,Gongxuan Lu. High Efficient Solar Hydrogen Generation by Modulation of Co-Ni Sulfide (220) Surface Structure and Adjusting Adsorption Hydrogen Energy. Applied Catalysis B: Environmental,2017,206,353−363.

[34] Bin Tian,Baojun Yang,Jian Li,Zhen Li,Wenlong Zhen,Yuqi Wu,Gongxuan Lu. Water Splitting by CdS/Pt/WO3-CeOx Photocatalysts with Assisting of Artificial Blood Perfluorodecalin. Journal of Catalysis,2017,350,189−196.

[35] Zhen Li,Bin Tian,Wenlong Zhen,Yuqi Wu and Gongxuan Lu. Inhibition of Hydrogen and Oxygen Recombination using Oxygen Transfer Reagent Hemin Chloride in Pt/TiO2 Dispersion for Photocatalytic Hydrogen Generation. Applied Catalysis B: Environmental,2017,203,408−415.

[36] Bin Tian,Wenlong Zhen,Haibo Gao,Xuqiang Zhang,Zhen Li,Gongxuan Lu. Carboxyl-assisted Synthesis of Co Nanorods with High Energy Facet on Graphene Oxide Sheets for Efficient Photocatalytic Hydrogen Evolution. Applied Catalysis B: Environmental,2017,203,789−797.

[37] Gongxuan Lu,Wenlong Zhen. Formation of Helium-3 and Helium-4 during Photocatalytic Hydrogen Generation over Cadmium Sulfide under Visible Light Irradiation. Journal of Molecular Catalysis(China),2017,31,299-304.

[38] Wenlong Zhen,Jiantai Ma,Gongxuan Lu. Small-Sized Ni(111) Particles in Metal-Organic Frameworks with Low Over-potential for Visible Photocatalytic Hydrogen Generation. Applied Catalysis B: Environmental,2016,190,12−25.

[39] Wenlong Zhen,Haibo Gao,Bin Tian,Jiantai Ma,Gongxuan Lu. Fabrication of Low Adsorption Energy Ni-Mo Cluster Cocatalyst in Metal-Organic Frameworks for Visible Photocatalytic Hydrogen Evolution. ACS Applied Materials & Interfaces,2016,8,10808–10819.

[40] Bin Tian,Zhen Li,Wenlong Zhen,Gongxuan Lu. Uniformly Sized (112) Facet Co2P on Graphene for Highly Effective Photocatalytic Hydrogen Evolution. Journal of Physical Chemistry C,2016,120,6409–6415.

[41] Bo Li,Wenlong Zhen,Gongxuan Lu,Jiantai Ma. The Adjustment of Product Distribution of CO2 Hydrogenation over Cu-Fe-Zn Catalyst while Maintaining its Activity via Potassium Addition. Journal of Molecular Catalysis(China),2015,29,152-163.

[42] Wenlong Zhen,Bo Li,Gongxuan Lu,Jiantai Ma. Enhancing Catalytic Activity and Stability for CO2 Methanation on Ni@MOF-5 via Control of Active Species Dispersion. Chemical Communications,2015,51,1728−1731.

[43] Wenlong Zhen,Bo Li,Gongxuan Lu,Jiantai Ma. Enhancing Catalytic Activity and Stability for CO2 Methanation on Ni–Ru/γ-Al2O3 via Modulating Impregnation Sequence and Controlling Surface Active Species. RSC Advances,2014,4,16472−16479.

[44] Yuanzhe Chen,Fengwei Zhang,Yiyun Fang,Xiaohang Zhu,Wenlong Zhen,Rou Wang,Jiantai Ma. Phosphotungstic acid containing ionic liquid immobilized on magnetic mesoporous silica rod catalyst for the oxidation of dibenzothiophene with H2O2. Catalysis Communications,2013,38,54-58.

联系方式:

电话:0931-4968062

地址:兰州市天水中路18号

邮箱:wlzhen@licp.cas.cn

未经中国科学院兰州化学物理研究所书面特别授权,请勿转载或建立镜像,违者依法必究